pp. 1-228 (April 2023)
pp. 1-200 (March 2023)
pp. 1-138 (February 2023)
pp. 1-144 (January 2023)
pp. 1-108 (December 2022)
pp. 1-106 (November 2022)
pp. 1-122 (October 2022)
pp. 1-124 (September 2022)
pp. 1-102 (August 2022)
pp. 1-112 (July 2022)
pp. 1-138 (June 2022)
pp. 1-186 (May 2022)
pp. 1-124 (April 2022)
pp. 1-104 (March 2022)
pp. 1-120 (February 2022)
pp. 1-124 (January 2022)
pp. 1-214 (June 2021)
pp. 1-90 (December 2021)
pp. 1-222 (April 2021)
pp. 1-324 (October 2021)
pp. 1-200 (February 2021)
pp. 1-222 (August 2021)
pp. 1-208 (December 2020)
pp. 1-112 (October 2020)
pp. 1-210 (August 2020)
pp. 1-204 (June 2020)
pp. 1-218 (April 2020)
pp. 1-182 (February 2020)
pp. 1-104 (December 2019)
pp. 1-116 (October 2019)
pp. 1-130 (August 2019)
pp. 1-224 (June 2019)
pp. 1-226 (April 2019)
pp. 1-216 (February 2019)
pp. 1-132 (December 2018)
pp. 1-182 (October 2018)
pp. 1-116 (August 2018)
pp. 1-228 (June 2018)
pp. 1-154 (April 2018)
pp. 1-198 (February 2018)
pp. 1-118 (December 2017)
pp. 1-162 (October 2017)
pp. 1-138 (August 2017)
pp. 1-190 (June 2017)
pp. 1-220 (April 2017)
pp. 1-164 (February 2017)
pp. 1-176 (December 2016)
pp. 1-138 (October 2016)
pp. 1-144 (August 2016)
pp. 1-122 (June 2016)
pp. 1-166 (April 2016)
pp. 1-222 (February 2016)
pp. 1-118 (December 2015)
pp. 1-194 (October 2015)
pp. 1-212 (August 2015)
pp. 1-150 (June 2015)
pp. 1-184 (April 2015)
pp. 1-200 (February 2015)
pp. 1-172 (December 2014)
pp. 1-230 (October 2014)
pp. 1-178 (August 2014)
pp. 1-138 (June 2014)
pp. 1-150 (April 2014)
pp. 1-122 (February 2014)
pp. 619-792 (December 2013)
pp. 475-618 (October 2013)
pp. 359-474 (August 2013)
pp. 249-358 (June 2013)
pp. 119-248 (April 2013)
pp. 1-118 (February 2013)
pp. 649-788 (December 2012)
pp. 523-647 (October 2012)
pp. 397-522 (August 2012)
pp. 255-396 (June 2012)
pp. 145-253 (April 2012)
pp. 1-143 (February 2012)
pp. 545-662 (December 2011)
pp. 451-544 (October 2011)
pp. 319-450 (August 2011)
pp. 193-317 (June 2011)
pp. 101-191 (April 2011)
pp. 1-99 (February 2011)
pp. 491-644 (December 2010)
pp. 399-489 (October 2010)
pp. 301-397 (August 2010)
pp. 187-299 (June 2010)
pp. 81-185 (April 2010)
pp. 1-80 (February 2010)
pp. 421-512 (December 2009)
pp. 337-419 (October 2009)
pp. 231-335 (August 2009)
pp. 161-229 (June 2009)
pp. 93-160 (April 2009)
pp. 1-91 (February 2009)
pp. 389-583 (December 2008)
pp. 289-388 (October 2008)
pp. 225-288 (August 2008)
pp. 131-222 (June 2008)
pp. 59-129 (April 2008)
pp. 1-58 (February 2008)
pp. 363-428 (December 2007)
pp. 305-361 (October 2007)
pp. 247-304 (August 2007)
pp. 193-246 (June 2007)
pp. 1-191 (April 2007)
pp. 259-361 (December 2006)
pp. 211-258 (October 2006)
pp. 103-210 (July 2006)
pp. 47-102 (April 2006)
pp. 1-46 (February 2006)
pp. 289-404 (December 2005)
pp. 243-288 (October 2005)
pp. 197-242 (August 2005)
pp. 151-196 (June 2005)
pp. 1-150 (April 2005)
pp. 235-280 (December 2004)
pp. 189-234 (October 2004)
pp. 139-188 (August 2004)
pp. 93-138 (June 2004)
pp. 47-92 (April 2004)
pp. 1-46 (February 2004)
pp. 231-276 (December 2003)
pp. 185-230 (October 2003)
pp. 139-183 (September 2003)
pp. 93-138 (July 2003)
pp. 47-92 (June 2003)
pp. 1-46 (April 2003)
Partic. vol. 18 pp. 96-104 (February 2015) doi: 10.1016/j.partic.2013.10.003
PM2.5 and PM10-2.5 chemical composition and source apportionment near a Hong Kong roadway ☆
Yan Chenga, b, c, *, Shuncheng Leec, Zhaolin Gua, Kinfai Hod, Yunwei Zhanga, Yu Huangc, Judith C. Chowa, b, e, John G. Watsona, b, e, Junji Caob, Renjian Zhangf
Highlights
Abstract
Twenty-four-hour PM2.5 and PM10 samples were collected simultaneously at a highly trafficked roadside site in Hong Kong every sixth day from October 2004 to September 2005. The mass concentrations of PM2.5, PM10-2.5 (defined as PM10 − PM2.5), organic carbon (OC), elemental carbon (EC), water-soluble ions, and up to 25 elements were determined. Investigation of the chemical compositions and potential sources revealed distinct differences between PM2.5 and PM10-2.5. The annual average mass concentrations were 55.5 ± 25.5 and 25.9 ± 15.7 μg/m3 for PM2.5 and PM10-2.5, respectively. EC, OM (OM = OC × 1.4), and ammonium sulfate comprised over ∼82% of PM2.5, accounting for ∼29%, ∼27%, and ∼25%, respectively, of the PM2.5 mass. Low OC/EC ratios (less than 1) for PM2.5 suggested that fresh diesel-engine exhaust was a major contributor. Seven sources were resolved for PM2.5 by positive matrix factorization (PMF) model, including vehicle emissions (∼29%), secondary inorganic aerosols (∼27%), waste incinerator/biomass burning (∼23%), residual oil combustion (∼10%), marine aerosols (∼6%), industrial exhaust (∼4%), and resuspended road dust (∼1%). EC and OM comprised only ∼19% of PM10-2.5. The average OC/EC ratio of PM10-2.5 was 7.8 ± 14.2, suggesting that sources other than vehicular exhaust were important contributors. The sources for PM10-2.5 determined by the PMF model included ∼20% traffic-generated resuspension (e.g., tire dust/brake linear/petrol evaporation), ∼17% locally resuspended road dust, ∼17% marine aerosols, ∼12% secondary aerosols/field burning, and ∼11% vehicle emissions.
Graphical abstract
Keywords
PM2.5; PM10-2.5; Roadside; Chemical composition; Source apportionment; Hong Kong